Thursday 24 December 2015

Switch from Bloch to Nèel DWs


Analytic theory for the switch from Bloch to Néel domain wall in nanowires with perpendicular anisotropy
M. D. DeJong and K. L. Livesey
Phys. Rev. B 92, 214420 (2015)

(a) The geometry of a rectangular nanowire with perpendicular magnetic anisotropy, width w and thickness d. Arrows show the direction of magnetization. Depending on the size of w and d, the lowest energy domain wall may be of (b) Bloch or (c) Néel type. In the Bloch wall, the magnetization rotates perpendicular to the wire's long z axis, in the xy plane. In the Néel wall, the magnetization rotates along the wire's long z axis, in the yz plane.

Magnetization dynamics in individual magnetite nanocrystals

Probing magnetization dynamics in individual magnetite nanocrystals using magnetoresistive scanning tunneling microscopy.
Amir Hevroni, Boris Tsukerman, and Gil Markovich
Phys. Rev. B 92, 224423 (2015)
(a), (d), and (g) Current vs time measurements performed on the three particles. Each particle was examined at a different temperature (indicated on the figure). In the case of particle 3, the graph shown is one of five consecutive measurements. (b), (e), and (h) Constant current STM topography images of the three particles. (c), (f), and (i) Height profiles of the measured particles, which are marked by arrows.

Wednesday 23 December 2015

Small is Smarter: Nano MRI Contrast Agents – Advantages and Recent Achievements - Gao - 2015 - Small - Wiley Online Library

Small is Smarter: Nano MRI Contrast Agents – Advantages and Recent Achievements.

Zhenyu Gao, Tiancong Ma, Enyu Zhao, Dominic Docter, Wensheng Yang, Roland H. Stauber and Mingyuan Gao
Small 12, 556 (2015)

Magnetic nanoparticles hold great potential as contrast agents for magnetic resonance imaging and advanced applications in multimodality imaging and drug carriers for cancer thranostics. To promote the development of this field, state-of-the-art achievements are summarized and fundamental scientific challenges are discussed

Magnetization reversal of an individual exchange-biased permalloy nanotube

Magnetization reversal of an individual exchange-biased permalloy nanotube.
A. Buchter, R. Wölbing, M. Wyss, O. F. Kieler, T. Weimann, J. Kohlmann, A. B. Zorin, D. Rüffer, F. Matteini, G. Tütüncüoglu, F. Heimbach, A. Kleibert, A. Fontcuberta i Morral, D. Grundler, R. Kleiner, D. Koelle, and M. Poggio
Phys. Rev. B 92, 214432 (2015)
Training effect: (a) SQUID and (b) DCM hysteresis loops for different loop number n at T=3.4 K. Red and blue curves indicate up- and down-sweep, respectively. Evolution of (c) exchange field and (d) coercivity with increasing loop number n extracted from SQUID data set. Dashed line fits the data according to Eq. (2). Point size corresponds to the measurement error in field

Tuesday 22 December 2015

Chiral damping of DWs

Chiral damping of magnetic domain walls.

Emilie Jué, C. K. Safeer, Marc Drouard, Alexandre Lopez, Paul Balint, Liliana Buda-Prejbeanu, Olivier Boulle, Stephane Auffret, Alain Schuhl, Aurelien Manchon, Ioan Mihai Miron & Gilles Gaudin
Nature Materials AOL (2015)
Graphic illustration of the asymmetric DW dynamics in PMA materials.

Friday 18 December 2015

Fundamentals and advances in magnetic hyperthermia

Fundamentals and advances in magnetic hyperthermia.
E. A. Périgo, G. Hemery, O. Sandre, D. Ortega, E. Garaio, F. Plazaola and F. J. Teran
Appl. Phys. Rev. 2, 041302 (2015)
(a) 3D scatter plot showing the main experimental conditions reported in a set of 120 publications on MH spanning over the last 25 years. Scatter size is proportional to the product. Green dots of different intensities are the 2D projection of the central scatter over the XY, XZ, and YZ planes. The color code of the spheres is related to the type of assay described in the corresponding publication: red refers to tests, yellow to tests, blues to combined / tests, and cyan to measurements. The dashed black curve superimposed to the field intensity vs maximum frequency plane indicates the “Brezovich” or criterion, along which the  = 4.8 × 108 A(ms)−1 condition is fulfilled [note that the experiments complying with this criterion are those below the curve]. (b) Zoom of the most populated region of (a), where the concentration of measurements in the 2005–2009 period an tests in the 2010–2015 period is shown.
 


Classical and quantum dynamics of molecular spins on graphene

The classical and quantum dynamics of molecular spins on graphene.
Christian Cervetti, Angelo Rettori, Maria Gloria Pini, Andrea Cornia, Ana Repollés, Fernando Luis, Martin Dressel, Stephan Rauschenbach, Klaus Kern, Marko Burghard, Lapo Bogani
a, |msright fence sublevels of the ground state of the single-molecule-magnet [Fe4(L)2(dpm)6], as obtained from equation (1). Absorption of phonons allows the barrier to be thermically overcome (green arrows). W ± n indicate the transition probabilities between magnetic |mright fence states induced by the absorption (+) or emission (−) of n phonons. Quantum tunnelling happens between admixed levels (red arrows), whereas hyperfine and dipolar interactions create energy distributions (orange). Interaction with Dirac electrons increases the tunnel splittings below |3right fence and |−3right fence (red areas, exaggerated for clarity). b, Temperature and frequency dependence of the imaginary component of the dynamic susceptibility (χ′′) in a magnetic field H = 1kOe for [Fe4(L)2(dpm)6] (top) and hybrids with isolated molecules (bottom). Lines are simulations with the theory (see text for the theory). c, Temperature and frequency dependence of the real component of the dynamic susceptibility (χ′) in H = 0 for [Fe4(L)2(dpm)6] (top) and hybrids with isolated molecules (bottom). Lines are simulations with the theory (see text for the theory).



Sunday 13 December 2015

Origin of perpendicular anisotropy in Fe atoms

Origin of Perpendicular Magnetic Anisotropy and Large Orbital Moment in Fe Atoms on MgO.
S. Baumann, F. Donati, S. Stepanow, S. Rusponi, W. Paul, S. Gangopadhyay, I. G. Rau, G. E. Pacchioni, L. Gragnaniello, M. Pivetta, J. Dreiser, C. Piamonteze, C. P. Lutz, R. M. Macfarlane, B. A. Jones, P. Gambardella, A. J. Heinrich, and H. Brune

(a) STM image of two Fe atoms on a ML MgO(100) grown on Ag(100) (4nm×4nm, tunnel current It=5  pA, tunnel voltage Vt=100mV). (b) Side view of DFT-calculated binding geometry and charge density [color scale, 1e/(au)3; Fe, green; O, red; Mg, blue). (Middle sketch) Top view ball model of the binding geometry. (c) Oblique view of DFT-calculated valence electron spin density contours (positive spin polarization, red; negative, blue).

Spin-glass-like freezing of inner and outer surface layers in hollow γ-Fe2O3 nanoparticles

Spin-glass-like freezing of inner and outer surface layers in hollow γ-Fe2O3 nanoparticles.
Hafsa Khurshid, Paula Lampen-Kelley, Òscar Iglesias, Javier Alonso, Manh-Huong Phan, Cheng-Jun Sun, Marie-Louise Saboungi & Hariharan Srikanth
Snapshots of the outer and inner surface spin configurations subject to varying magnetic fields (a) h = 100 (the maximum positive applied field), (b) h = 0 (remanence at the upper branch), (c) h = −25 (near the negative coercive field), and (d) h = −100 (the maximum negative applied field). Spins have been colored with a gradient from dark-red/dark-blue (outer/inner surface) for spins along the field direction to yellow/green (outer/inner surface) for spins transverse to the field direction. Only a slice of the spin configurations of a hollow nanoparticle close to the central plane and perpendicular to the field direction is shown.

Hysteresis of quantum uniaxial superparamagnets

Nonlinear ac stationary response and dynamic magnetic hysteresis of quantum uniaxial superparamagnets.

Yuri P. Kalmykov, Serguey V. Titov, and William T. Coffey

Phys. Rev. B 92, 174414 (2015)

DMH loops [m(t)=SˆZ(t)/S vs h(t)=cosωt] for various anisotropy parameters σ=10 (a), 15 (b), 20 (c), and various spin numbers S=3/2 (1: short-dashed lines), 4 (2: solid lines), 10 (3: dashed-dotted lines), 20 (4: dashed lines), and (asterisks) at ωτN=104, ξ0=0, and ξ=9.

Saturday 12 December 2015

A magnetic protein biocompass

A magnetic protein biocompass.
Siying Qin, Hang Yin, Celi Yang, Yunfeng Dou, Zhongmin Liu, Peng Zhang, He Yu, Yulong Huang, Jing Feng, Junfeng Hao, Jia Hao, Lizong Deng, Xiyun Yan, Xiaoli Dong, Zhongxian Zhao, Taijiao Jiang, Hong-Wei Wang, Shu-Jin Luo & Can Xie
Nature Materials 15,217 (2016)
The biocompass model of animal magnetoreception and navigation.


Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes : Nature Communications : Nature Publishing Group

Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes.
Yoann Prado, Niéli Daffé, Aude Michel, Thomas Georgelin, Nader Yaacoub, Jean-Marc Grenèche, Fadi Choueikani, Edwige Otero, Philippe Ohresser, Marie-Anne Arrio, Christophe Cartier-dit-Moulin, Philippe Sainctavit, Benoit Fleury, Vincent Dupuis, Laurent Lisnard, Jérôme Fresnais
(a) Field-cooled and zero-field-cooled (FC/ZFC) magnetization curves measured in the 5–80K temperature range under an applied field of 50Oe and (b) magnetization vs field curves measured at 5K for 0b and 1 in diluted solutions.


Tuesday 8 December 2015

Criteria for saturated magnetization loop

Criteria for saturated magnetization loop.

A. Harres, M. Mikhov, V. Skumryev, A.M.H. de Andrade, J.E. Schmidt, J. Geshev

J. Magn. Magn. Mater.402, 76 (2015)

M(H  ) loops calculated for a disordered system of non-interacting single-domain uniaxial-anisotropy particles using View the MathML source, where View the MathML source (panel (a)) and View the MathML source (panel (b)). The first (panels (c) and (d)) and the second (panels (e) and (f)) derivatives of the respective descending and ascending branches for negative fields are also given. Although View the MathML source for both loops and their derivatives, only the regions of interest are plotted. The bottom panels show the −md(H) and mr(H) (the latter obtained starting from a random magnetization state) remanence curves; the first derivatives of −md(H) are plotted in the insets.

Friday 4 December 2015

Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes : Nature Communications : Nature Publishing Group

Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes.
Yoann Prado, Niéli Daffé, Aude Michel, Thomas Georgelin, Nader Yaacoub, Jean-Marc Grenèche, Fadi Choueikani, Edwige Otero, Philippe Ohresser, Marie-Anne Arrio, Christophe Cartier-dit-Moulin, Philippe Sainctavit, Benoit Fleury, Vincent Dupuis, Laurent Lisnard; Jérôme Fresnais
Nature Communications 6, 10139 (2015)
(a) Representation of the [Co(TPMA)Cl2] complex used to enhance the magnetic anisotropy of the γ-Fe2O3 nanoparticles. (b) TEM image of the γ-Fe2O3 nanoparticles functionalized with the cobalt(II) complex: 1 (5.0nm, σ=0.09) and (c) schematic view of the coordination of the complex with the iron ions. (d) Synthesis scheme with measured pH values, hydrodynamic diameters (Zav), sizes (D) and distributions (σ).
Tuning the magnetic anisotropy in coordination nanoparticles: random distribution versus core–shell architecture.
Yoann Prado, Nada Dia, Laurent Lisnard, Guillaume Rogez, François Brisset, Laure Catala and   Talal Mallah

Core–shell magnetic coordination nanoparticles made of a soft core and a hard magnetic shell, containing anisotropic Co(II) ions, display a dramatic increase in their average blocking temperature with a coercive field value 25 times larger than that of the soft core, due to a large enhancement of the magnetic anisotropy.